Abstract
[Objective] To investigate the factors affecting the extraction rate, characteristic aroma components, and stability of Phyllanthus emblica L.extracts from different producing areas. [Methods] Five types of P.emblica from four producing areas, including Guangdong, Yunnan, Jiangxi, and Sichuan, were used as raw materials.Orthogonal experiments were conducted to study the effects of various factors on the extraction rate.Gas chromatography -mass spectrometry (GC-MS) analysis and similarity calculations were used to compare the characteristic aroma components of P.emblica extracts from different producing areas.The stability of the extracts was evaluated based on appearance, relative density, and sugar content. [Results] Among the producing areas, dried P.emblica from Yunnan had the highest extraction rate, with solvent and material -to-liquid ratio being the main factors influencing extraction.GC -MS analysis showed that characteristic aroma components of extracts from Guangdong included furfural, furfuralcohol, pyranone, 5-hydroxymethylfurfural, and ethyl palmitate, whereas extracts from Yunnan were characterized by 3-methyl -2-furanic acid and dibutyl phthalate.The similarity between these two extracts was only 0.943 6. [Conclusion] All five P.emblica extracts exhibited a prominent fruity -sweet aroma.However, there were significant differences in characteristic aroma components among different producing areas and varieties.The extracts also demonstrated good preservation and usage stability over a certain period.
Publication Date
12-11-2025
First Page
20
Last Page
27
DOI
10.13652/j.spjx.1003.5788.2025.80026
Recommended Citation
Rui, LI; Hongyou, HUANG; Jie, MAO; Wenbo, ZHAO; Mingqin, ZHAO; and Juncang, PENG
(2025)
"Extraction of characteristic aroma components from Phyllanthus emblica L. and analysis of its stability,"
Food and Machinery: Vol. 41:
Iss.
11, Article 3.
DOI: 10.13652/j.spjx.1003.5788.2025.80026
Available at:
https://www.ifoodmm.cn/journal/vol41/iss11/3
References
[1] 李雪冬,潘烨华,田雨闪,等.余甘子的本草考证及其现代研究中若干问题的探讨 [J].中草药,2022,53(18):5 873-5 883.LI X D,PAN Y H,TIAN Y S,et al.Herbal textual and key problems in modern research of Phyllanthus emblica [J].Chinese Traditional and Herbal Drugs,2022,53(18):5 873-5 883.
[2] 杨婉媛,陈晓维,刘杜娟,等.余甘子的生物活性及加工研究进展 [J].广东农业科学,2022,49(7):120-130.YANG W Y,CHEN X W,LIU D J,et al.Research progress in biological activity and processing of Phyllanthus emblica [J].Guangdong Agricultural Sciences,2022,49(7):120-130.
[3] 唐春红,陈冬梅,陈岗,等.余甘子果实提取物活性成分分离及结构鉴定 [J].食品科学,2009,30(9):103-108.TANG C H,CHEN D M,CHEN G,et al.Isolation and structural identification of antibacterial components from Phyllanthus emblica L.[J].Food Science,2009,30(9):103-108.
[4] 刘 晓 晖,吕 乔,吉 雄,等.余 甘 子 化 学 成 分 研 究 [J].中 成 药,2023,45(2):458-462.LIU X H,LÜ Q,JI X,et al.Chemical constituents from Phyllanthus emblica [J].Chinese Traditional Patent Medicine,2023,45(2):458-462.
[5] 张沐棠,陈少虹,程子贤,等.余甘子的回甘风味研究进展 [J].食品与发酵工业,2023,49(6):324-331.ZHANG M T,CHEN S H,CHENG Z X,et al.Research development of the back sweet flavour of Phyllanthus emblica L.[J].Food and Fermentation Industries,2023,49(6):324-331.
[6] 兰杨,姜红,张仕瑾,等.余甘子化学成分、药理活性及质量控制提升的研究进展 [J].中国药业,2020,29(7):156-159.LAN Y,JIANG H,ZHANG S J,et al.Research progress on chemical constituents,pharmacological activities and quality control of Phyllanthus emblica [J].China Pharmaceuticals,2020,29(7):156-159.
[7] YANG F,YASEEN A,CHEN B,et al.Chemical constituents from the fruits of Phyllanthus emblica L[J].Biochemical Systematics and Ecology,2020,92:104122.
[8] GUL M,LIU Z W,IAHTISHAM-UL-HAQ,et al.Functional and nutraceutical significance of amla (Phyllanthus emblica L.):a review [J].Antioxidants,2022,11(5):816.
[9] 陈静梅,郝二伟,杜正彩,等.基于化学成分、药理作用和网络药理学的余甘子质量标志物 (Q-Marker )预测分析 [J].中草药,2022,53(5):1 570-1 586.CHEN J M,HAO E W,DU Z C,et al.Predictive analysis on quality marker of Phyllanthus emblica based on chemical composition,pharmacological effects and network pharmacology [J].Chinese Traditional and Herbal Drugs,2022,53(5):1 570-1 586.
[10] AHMAD B,HAFEEZ N,RAUF A,et al.Phyllanthus emblica:a comprehensive review of its therapeutic benefits [J].South African Journal of Botany,2021,138:278-310.
[11] WANG S H,GUO C,CUI W J,et al.Two pyrrole acids isolated from Phyllanthus emblica L.and their bioactivities [J].Natural Products and Bioprospecting,2023,13(1):26.
[12] 刘 晓 丽,杨 冰 鑫,陈 柳 青,等.HPLC 测 定 余 甘 子 茶 中 3种 多酚 成 分 及 抗 氧 化 活 性 研 究 [J].食 品 工 业 科 技,2020,41(13):315-320,327.LIU X L,YANG B X,CHEN L Q,et al.Determination of three polyphenol components in Phyllanthus emblica L.tea by high performance liquid chromatography and their antioxidant activity [J].Science and Technology of Food Industry,2020,41(13):315-320,327.
[13] 叶 烨,李 东 亮,耿 宗 泽,等.基 于 AB-8大 孔 吸 附 树 脂 制 备 余甘 子 果 实 精 制 物 及 其 在 卷 烟 中 的 应 用 [J].烟 草 科 技,2021,54(2):52-57.YE Y,LI D L,GENG Z Z,et al.Preparation and refinement of Phyllanthus emblica extract on macroporous resins and its application to cigarettes [J].Tobacco Science & Technology,2021,54(2):52-57.
[14] LI R,YANG J C,YIN X Q,et al.Thermal pyrolysis of two synthesized Amadori derivatives prepared by protecting the active groups [J].Journal of Analytical and Applied Pyrolysis,2024,177:106351.
[15] 杨金初,孙世豪,胡军,等.以天然植物水提取物为美拉德反应原料制备天然香料 [J].烟草科技,2017,50(12):44-54.YANG J C,SUN S H,HU J,et al.Natural flavor preparation via Maillard reaction of plant water extracts [J].Tobacco Science & Technology,2017,50(12):44-54.
[16] 龙小妹,李蓉,郭爽,等.余甘子鲜果不同部位中 7种有效成分的含量比较 [J].医药导报,2024,43(5):785-790.LONG X M,LI R,GUO S,et al.Comparison of the content of seven active ingredients in different parts of the fresh fruit of Phyllanthus emblica [J].Herald of Medicine,2024,43(5):785-790.
[17] DENBAUM E,ALTERN S H,VECCHIARELLO N,et al.A batch screening technique for the calculation of chromatographic separability [J].Journal of Chromatography A,2024,1 732:465170.
[18] 马宇平,席高磊,赵志伟,等.香气活性值用于许昌、郴州和潍坊烤烟香气差异分析 [J].烟草科技,2020,53(5):63-70.MA Y P,XI G L,ZHAO Z W,et al.Analysis of aroma differences of flue-cured tobacoo leaves from Xuchang,Chenzhou and Weifang based on aroma activity values [J].Tobacco Science & Technology,2020,53(5):63-70.
[19] 李晓强,胡坤,龚玉石,等.不同产地、不同提取方法对余甘子 多 酚 含 量 及 抗 氧 化 活 性 的 影 响 [J].食 品 工 业 科 技,2023,44(2):317-323.LI X Q,HU K,GONG Y S,et al.Effects of different producing areas and extraction methods of polyphenols from Phyllanthus emblica L.[J].Science and Technology of Food Industry,2023,44(2):317-323.
[20] 夏念桐,路娟,李书洋,等.响应面法优化余甘子中多酚快速提取工艺 [J].食品工业,2024,45(4):127-131.XIA N T,LU J,LI S Y,et al.Optimization on the rapid extraction process of polyphenols from Phyllanthus emblica L.by response surface method [J].The Food Industry,2024,45(4):127-131.
[21] ZHANG G W,HU M M,HE L,et al.Optimization of microwave-assisted enzymatic extraction of polyphenols from waste peanut shells and evaluation of its antioxidant and antibacterial activities in vitro [J].Food and Bioproducts Processing,2013,91(2):158-168.
[22] 吴佳欣,周波,邓萌萌,等.加热时间对余甘子水煎液中没食子酸的影响 [J].中成药,2020,42(3):702-708.WU J X,ZHOU B,DENG M M,et al.Effects of heating time on gallic acid in the aqueous decoction of Phyllanthus emblica[J].Chinese Traditional Patent Medicine,2020,42(3):702-708.
[23] GUO X Y,HO C T,SCHWAB W,et al.Effect of the roasting degree on flavor quality of large-leaf yellow tea [J].Food Chemistry,2021,347:129016.
[24] DU J Y,LI Y M,XU J C,et al.Characterization of key odorants in Langyatai Baijiu with Jian flavour by sensory-directed analysis [J].Food Chemistry,2021,352:129363.
[25] 亓旗,崔雅萍,梁文仪,等.多指标正交试验法优选余甘子总酚提取工艺 [J].世界科学技术—中医药现代化,2017,19(9):1 544-1 548.QI Q,CUI Y P,LIANG W Y,et al.Optimum extraction technology of total polyphenol from Phyllanthus emblica via multi-target orthogonal design [J].Modernization of Traditional Chinese Medicine and Materia Medica-World Science and Technology,2017,19(9):1 544-1 548.
[26] 林 翔 云.香 料 香 精 辞 典 [M].北 京:化 学 工 业 出 版 社,2007:188,235.LIN X Y.Dictionary of flavor & fragrance [M].Beijing:Chemical Industry Press,2007:188,235.
[27] ZHU J C,XIAO Z B.Characterization of the major odor-active compounds in dry jujube cultivars by application of gas chromatography-olfactometry and odor activity value [J].Journal of Agricultural and Food Chemistry,2018,66(29):7 722-7 734.
[28] ZHU J C,WANG L Y,XIAO Z B,et al. Characterization of the key aroma compounds in mulberry fruits by application of gas chromatography-olfactometry (GC-O ),odor activity value (OAV ),gas chromatography-mass spectrometry (GC-MS ) and flame photometric detection (FPD ) [J].Food Chemistry,2018,245:775-785.
[29] 赵爱秀,邓泽元.亚麻籽油中酚类物质对亚麻籽油氧化稳定性的影响 [J].食品科技,2024,49(8):185-191.ZHAO A X,DENG Z Y.Effect of phenolic compounds in flaxseed oil on oxidative stability of flaxseed oil [J].Food Science and Technology,2024,49(8):185-191.
